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Hybrid Nanocrystals of Small Molecules and Chemically Disordered Polymers. Dannenhoffer, Hiroaki Sai, Jacob Kupferberg, Liam C. Bruckner, Tine Curk, Luka Đorđević, Ziwei Wang, Yang Yang, Ruomeng Qiu, Adam J. Journal of the American Chemical Society 2022, 144 AIE-Active, Stimuli-Responsive Fluorescent 2D Block Copolymer Nanoplatelets Based on Corona Chain Compression.

Shixing Lei, Jia Tian, Yuetong Kang, Yifan Zhang, Ian Manners.Frame Shifts Affect the Stability of Collagen Triple Helices. Barros, Marc-Olivier Ebert, Enrico Ruijsenaars, Sereina Riniker, Helma Wennemers. Journal of the American Chemical Society 2022, Article ASAP.

Scalable and Uniform Length-Tunable Biodegradable Block Copolymer Nanofibers with a Polycarbonate Core via Living Polymerization-Induced Crystallization-Driven Self-assembly.

This article is cited by 26 publications. Altogether, we establish a robust platform for constructing multifunctional 2D nanoarchitectures in which one can systematically program their compositional, spatial, and functional properties, which is a significant step toward their deployment into functional nanoscale devices. Finally, we demonstrate that different sectors of the sheet surface can be selectively functionalized using bioorthogonal conjugation chemistry. Structural information, gathered from SAXS and cryo-TEM, reveals that the distinct peptide domains maintain their intrinsic lattice structure and illuminates various mechanisms employed by CMP triple helices to alleviate the elastic strain associated with the interfacial lattice mismatch. Modulating their thermodynamic stability affords the controlled synthesis of 2D core–shell nanostructures via thermally driven heteroepitaxial growth. Collagen triple helices, comprising collagen-mimetic peptides (CMPs), are employed as molecularly programmable crystallizable units. Herein, we demonstrate a straightforward strategy for the thermodynamically controlled fabrication of multicomponent sectored nanosheets in which each sector can be chemically and spatially addressed independently and orthogonally. Engineering free-standing 2D nanomaterials with compositional, spatial, and functional control across size regimes from the nano- to mesoscale represents a significant challenge.

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